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Sasa, Toshinobu
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.211 - 215, 2022/05
Lead-bismuth eutectic (LBE) alloy is promising as a spallation target for next-generation reactor coolants and accelerator drive systems (ADS) due to its nuclear and chemical properties. LBE is a heavy metal, and it has good properties both as a spallation target and as a coolant for nuclear transmutation systems of long-lived radioactive nuclei. On the other hand, to improve compatibility with structural materials is one of the major issues in its utilization. The latest research results such as high-temperature operation of LBE and oxygen concentration control to ensure corrosion resistance with the aim of early commercialization of nuclear conversion technology by ADS is introduced.
Obayashi, Hironari; Yamaki, Kenichi*; Yoshimoto, Hidemitsu*; Kita, Satoshi*; Wan, T.*; Sasa, Toshinobu
JAEA-Technology 2021-035, 66 Pages, 2022/03
JAEA-Technology-2021-035.pdf:4.26MB
Construction of Transmutation Experimental Facility (TEF) is under planning in Japan Proton Accelerator Research Complex (J-PARC) program to promote R&Ds on realization of transmutation technology by an accelerator driven system (ADS). As a facility of TEF, ADS Target Test Facility (TEF-T) will provide a spallation target to study target technology and perform post irradiation examination (PIE) of candidate materials of ADS. In ADS, lead-bismuth eutectic (LBE) alloy is used as a spallation target material and a core coolant. As is well known, LBE has corrosive to structural materials hence each component of the target system should provide compatibility with LBE. In addition, instrumentations for LBE are restricted by the target operation condition such as high temperature and irradiation environment. The devices for LBE have been developed individually to achieve the LBE target system. "Integrated Multi-functional MOckup for TEF-T Real-scale TArget Loop, IMMORTAL" was fabricated as a mock-up test loop of the target for the purpose of the integration testing of individually developed devices. This report describes an overview of IMMORTAL and the design of the installed devices.
Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
Journal of Nuclear Science and Technology, 57(10), p.1141 - 1151, 2020/10
Times Cited Count：11 Percentile：75.12(Nuclear Science & Technology)To estimate the structural damages of materials in accelerator facilities, displacement per atom (dpa) is widely employed as a damage index, calculated based on the displacement cross-section obtained using a calculation model. Although dpa is applied as standard, the experimental data of the displacement cross-section for a proton in the energy region above 20 MeV are scarce. Among the calculation models, difference of about factor 8 exist, so that the experimental data of the cross-section are crucial to validate the model. To obtain the displacement cross-section, we conducted experiments at J-PARC. The displacement cross-section of copper and iron was successfully obtained for a proton projectile with the kinetic energies, 0.4 - 3 GeV. The results were compared with those obtained using the widely utilized Norgertt-Robinson-Torrens (NRT) model and the athermal-recombination-corrected (arc) model based on molecular dynamics. It was found that the NRT model overestimates the present displacement cross-section by 3.5 times. The calculation results obtained using with the arc model based on the Nordlund parameter show remarkable agreement with the experimental data. It can be concluded that the arc model must be employed for the dpa calculation for the damage estimation of copper and iron.
Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Maekawa, Fujio; Matsuda, Hiroki; Sasa, Toshinobu; Meigo, Shinichiro
Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10
Times Cited Count：5 Percentile：48.18(Nuclear Science & Technology)Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350
C to 500C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Rb, Tl, Tc, Os, Ir, Pt, Au and Hg were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Sr, Zr and Y were stable as CeO
, SrO, ZrO and YO
in the LBE.
Wan, T.; Obayashi, Hironari; Sasa, Toshinobu
Nuclear Technology, 205(1-2), p.188 - 199, 2019/01
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)Kai, Tetsuya; Uchida, Toshitsugu; Kinoshita, Hidetaka; Seki, Masakazu; Oi, Motoki; Wakui, Takashi; Haga, Katsuhiro; Kasugai, Yoshimi; Takada, Hiroshi
Journal of Physics; Conference Series, 1021(1), p.012042_1 - 012042_4, 2018/06
Times Cited Count：0 Percentile：0.11(Nuclear Science & Technology)Maekawa, Fujio; Transmutation Expeimental Facility Design Team
Plasma and Fusion Research (Internet), 13(Sp.1), p.2505045_1 - 2505045_4, 2018/05
The partitioning and transmutation (P-T) technology has promising potential for volume reduction and mitigation of degree of harmfulness of high-level radioactive waste. JAEA is promoting development of the P-T technology by using an accelerator driven system (ADS). To facilitate the development, we have a plan to construct the Transmutation Experimental Facility (TEF) as one of experimental facilities of J-PARC (Japan Proton Accelerator Research Complex). TEF consists of two facilities: the ADS Target Test Facility (TEF-T) and the Transmutation Physics Experimental Facility (TEF-P). Recent progress in design and R&D efforts toward construction of J-PARC TEF will be presented.
Takada, Hiroshi; Haga, Katsuhiro; Teshigawara, Makoto; Aso, Tomokazu; Meigo, Shinichiro; Kogawa, Hiroyuki; Naoe, Takashi; Wakui, Takashi; Oi, Motoki; Harada, Masahide; et al.
Quantum Beam Science (Internet), 1(2), p.8_1 - 8_26, 2017/09
At the Japan Proton Accelerator Research Complex (J-PARC), a pulsed spallation neutron source provides neutrons with high intensity and narrow pulse width to promote researches on a variety of science in the Materials and life science experimental facility. It was designed to be driven by the proton beam with an energy of 3 GeV, a power of 1 MW at a repetition rate of 25 Hz, that is world's highest power level. A mercury target and three types of liquid para-hydrogen moderators are core components of the spallation neutron source. It is still on the way towards the goal to accomplish the operation with a 1 MW proton beam. In this paper, distinctive features of the target-moderator-reflector system of the pulsed spallation neutron source are reviewed.
Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Sugawara, Takanori; Wan, T.; Yamaguchi, Kazushi*; Yoshimoto, Hidemitsu
NEA/CSNI/R(2017)2 (Internet), p.111 - 116, 2017/06
Japan Atomic Energy Agency (JAEA) proposes to reduce the environmental impact caused from high-level radioactive waste by using Accelerator-driven system (ADS). To realize ADS, JAEA plans to build the Transmutation Experimental Facility (TEF) within the framework of J-PARC project. For the JAEA-proposed ADS, lead-bismuth eutectic alloy (LBE) is adopted as a coolant for subcritical core and spallation target. By using TEF in J-PARC, we are planning to solve technical difficulties for LBE utilization by completion of the data for the design of ADS. The 250kW LBE spallation target will be located in TEF facility to prepare material irradiation database. Various R&Ds for important technologies required to build the facilities are investigated such as oxygen content control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for 250kW target mock up and material corrosion studies are also manufactured and ready for various experiments. The latest status of 250kW LBE spallation target optimization will be described in the presentation.
Iwamoto, Hiroki; Nishihara, Kenji; Iwamoto, Yosuke; Hashimoto, Shintaro; Matsuda, Norihiro; Sato, Tatsuhiko; Harada, Masahide; Maekawa, Fujio
Journal of Nuclear Science and Technology, 53(10), p.1585 - 1594, 2016/10
Times Cited Count：18 Percentile：85.45(Nuclear Science & Technology)Sasa, Toshinobu; Takei, Hayanori; Saito, Shigeru; Obayashi, Hironari; Nishihara, Kenji; Sugawara, Takanori; Iwamoto, Hiroki; Yamaguchi, Kazushi; Tsujimoto, Kazufumi; Oigawa, Hiroyuki
NEA/CSNI/R(2015)2 (Internet), p.85 - 91, 2015/06
Nuclear transmutation got much interested as an effective option of nuclear waste management. Japan Atomic Energy Agency (JAEA) proposes the transmutation of minor actinides (MA) by accelerator-driven system (ADS) using lead-bismuth alloy (Pb-Bi). To obtain the data for ADS design, JAEA plans to build a Transmutation Experimental Facility (TEF) in the J-PARC project. TEF consists of two buildings, an ADS target test facility (TEF-T) with 400MeV-250kW Pb-Bi target, and a Transmutation Physics Experimental Facility (TEF-P), which set up a fast critical assembly driven by low power proton beam with MA fuel. In TEF-T, irradiation test for materials, and engineering tests for Pb-Bi target operation will be performed. Various research plans such as nuclear data measurements have been proposed and layout of the experimental hall are underway. In the presentation, roadmap to establish the ADS transmutor and latest design activities for TEF construction will be summarized.
Oigawa, Hiroyuki; Sasa, Toshinobu; Kikuchi, Kenji; Nishihara, Kenji; Kurata, Yuji; Umeno, Makoto*; Tsujimoto, Kazufumi; Saito, Shigeru; Futakawa, Masatoshi; Mizumoto, Motoharu; et al.
Proceedings of 4th International Workshop on the Utilisation and Reliability of High Power Proton Accelerators, p.507 - 517, 2005/11
Under the framework of J-PARC, the Japan Atomic Energy Research Institute (JAERI) plans to construct the Transmutation Experimental Facility (TEF). The TEF consists of two facilities: the Transmutation Physics Experimental Facility (TEF-P) and the ADS Target Test Facility (TEF-T). The TEF-P is a critical facility which can accept a 600 MeV - 10 W proton beam. The TEF-T is a material irradiation facility using a 600 MeV - 200 kW proton beam, where a Pb-Bi target is installed, but neutron multiplication by nuclear fuel will not be attempted. This report describes the purposes of the facility, the present status of the conceptual design, and the expected experiments to be performed.
Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Nishihara, Kenji; Saito, Shigeru; Mizumoto, Motoharu; Takano, Hideki*; et al.
Proceedings of 4th International Workshop on the Utilisation and Reliability of High Power Proton Accelerators, p.325 - 334, 2005/11
The Japan Atomic Energy Research Institute (JAERI) is conducting the research and development (R&D) on the Accelerator-Driven Subcritical System (ADS) for the effective transmutation of minor actinides (MAs). The ADS proposed by JAERI is the 800 MWth, Pb-Bi cooled, tank-type subcritical reactor loaded with (MA+Pu) nitride fuel. The Pb-Bi is also used as the spallation target. In this study, the feasibility of the ADS was discussed with putting the focus on the design around the beam window. The partition wall was placed between the target region and the ductless-type fuel assemblies to keep the good cooling performance for the hot-spot fuel pin. The flow control nozzle was installed to cool the beam window effectively. The thermal-hydraulic analysis showed that the maximum temperature at the outer surface of the beam window could be repressed below 500 C even in the case of the maximum beam power of 30 MW. The stress caused by the external pressure and the temperature distribution of the beam window was also below the allowable limit.
C and 550CKurata, Yuji; Futakawa, Masatoshi; Saito, Shigeru
JAERI-Research 2005-002, 37 Pages, 2005/02
JAERI-Research-2005-002.pdf:20.04MB
Static corrosion tests of various austenitic and ferritic/martensitic steels were conducted in oxygen-saturated liquid Pb-Bi at 450C and 550C for 3000h to study the effects of temperature and alloying elements on corrosion behavior. Oxidation, grain boundary corrosion, dissolution and penetration were observed. The corrosion depth decreases at 450C with increasing Cr content in steels regardless of ferritic/martensitic or austenitic steels. Appreciable dissolution of Ni and Cr does not occur in the three austenitic steels at 450C. The corrosion depth of ferritic/martensitic steels also decreases at 550C with increasing Cr content whereas the corrosion depth of austenitic steels, JPCA and 316ss becomes larger due to ferritization caused by dissolution of Ni at 550C than that of ferritic/martensitic steels. An austenitic stainless steel containing about 5%Si exhibits fine corrosion resistance at 550C because the protective Si oxide film is formed and prevents dissolution of Ni and Cr.
Oigawa, Hiroyuki; Tsujimoto, Kazufumi; Kikuchi, Kenji; Kurata, Yuji; Sasa, Toshinobu; Umeno, Makoto*; Saito, Shigeru; Nishihara, Kenji; Mizumoto, Motoharu; Takano, Hideki*; et al.
EUR-21227 (CD-ROM), p.483 - 493, 2005/00
JAERI is conducting the study on the dedicated transmutation system using the accelerator driven subcritical system (ADS). A subcritical reactor with the thermal power of 800 MW has been proposed. Many research and development activities including the conceptual design study are under way and planned at JAERI to examine the feasibility of the ADS. In the field of the proton accelerator, a superconducting LINAC is being developed. In the field of the spallation target using lead-bismuth eutectic (LBE), material corrosion, thermal-hydraulics, polonium behavior, and irradiation effect on materials are being studied. Moreover, in the framework of the J-PARC project, JAERI plans to construct the Transmutation Experimental Facility (TEF) to study the feasibility of the ADS using a high-energy proton beam and nuclear fuel and to establish the technology for the LBE spallation target and relevant materials.
Kurata, Yuji; Futakawa, Masatoshi; Saito, Shigeru
Journal of Nuclear Materials, 335(3), p.501 - 507, 2004/12
Times Cited Count：32 Percentile：85.88(Materials Science, Multidisciplinary)Corrosion tests were performed in oxygen-saturated liquid Pb-Bi at 450C and 550C in a pot for 3000h for Al-surface-treated steels containing various levels of Cr contents. The Al surface treatments were achieved using a gas diffusion method and a melt dipping method. AlO, FeAl and AlCr produced by the gas diffusion method exhibited corrosion resistance to liquid Pb-Bi, while the surface layer produced by the melt dipping method suffered a severe corrosion attack. Fe
Al
and FeAl
produced by the melt dipping method disappeared during the corrosion test at 550C and only FeAl remained.
Futakawa, Masatoshi; Naoe, Takashi*; Kogawa, Hiroyuki; Ikeda, Yujiro
Journal of Nuclear Science and Technology, 41(11), p.1059 - 1064, 2004/11
Times Cited Count：12 Percentile：61.44(Nuclear Science & Technology)High power spallation targets for neutron sources are developing in the world. Mercury target will be installed at the material and life science facility in J-PARC, which will promote innovative science. The mercury target is subject to the pressure wave caused by the proton bombarding mercury. The pressure wave propagation induces the cavitation in mercury that imposes localized impact damage on the target vessel. The impact erosion is a critical issue to decide the lifetime of the target. The electric Magnetic Impact Testing Machine, MIMTM, was developed to produce the localized impact erosion damage and evaluate the damage formation. Acoustic vibration measurement was carried out to investigate the correlation between damage and acoustic vibration. It was confirmed that the acoustic vibration is useful to predict the damage due to the localized impact erosion and to diagnose the structural integrity.
Kurata, Yuji; Futakawa, Masatoshi
Journal of Nuclear Materials, 325(2-3), p.217 - 222, 2004/09
Times Cited Count：37 Percentile：89.62(Materials Science, Multidisciplinary)The corrosion properties of three austenitic steels with different Si contents were studied under oxygen-saturated liquid Pb-Bi condition for 3000h. The three austenitic steels did not exhibit appreciable dissolution of Ni and Cr at 450C. At 550C, the thick ferrite layer produced by dissolution of Ni and Cr was found in JPCA and 316ss with low Si contents while the protective oxide film composed of Si and O was formed on 18Cr-20Ni-5Si steel and prevented dissolution of Ni and Cr. It was found that the Si added austenitic steel exhibited excellent corrosion resistance in liquid Pb-Bi.
Kinoshita, Hidetaka; Haga, Katsuhiro; Kaminaga, Masanori; Hino, Ryutaro
Journal of Nuclear Science and Technology, 41(3), p.376 - 384, 2004/03
Times Cited Count：3 Percentile：23.51(Nuclear Science & Technology)A construction of the spallation neutron source is being promoted under the Japan Proton Accelerator Research Complex (J-PARC) Project. A mercury circulation system has been designed to supply mercury to the target stably. It was necessary to make clear a mercury pump performance, erosion rate under the mercury flowing condition and an amount of remaining mercury after draining from the viewpoints of evaluating lifetime of piping and establishing remote handling scenario of mercury components. The mercury pump performance, the erosion rates and the amount of remained mercury were investigated by using a mercury experimental loop with an experimental gear pump. The discharged flow rates of the experimental gear pump are sufficient and it is increased linearly with the rotation speed. Erosion rates were found to be so small that decrease of piping wall thickness would be estimated 660 
m after 30-year operation under the rated velocity of 0.7 m/s. For the amount of remaining mercury, remaining rates of weight was estimated at 50.7 g/m
.
Haga, Katsuhiro; Kaminaga, Masanori; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Sato, Hiroshi; Ishikura, Shuichi*; Torii, Yoshikatsu; Hino, Ryutaro
Proceedings of 12th International Conference on Nuclear Engineering (ICONE-12) (CD-ROM), 8 Pages, 2004/00
In the Material and Life Science Facility, which will be constructed in the J-PARC project, the spallation mercury target station will be installed. Once the target system operation starts, mercury, the target vessel and the surrounding components are highly irradiated, so that all the replacement and maintenance operations of the target vessel and its peripheral devices have to be done with remote handling. In order to meet the requirements, we designed the target system such that the target vessel and the mercury circulation system are mounted on a target trolley, which is the system carriage. The target vessel is carried with the mercury circulation system together and inserted into the target center by the target trolley during the on-beam operation. During the system maintenance period, the target trolley is withdrawn to the maintenance room of hot cell, and the component exchange or repairing work will be done using a power manipulator and some master-slave manipulators. In this paper, the present design of the mercury target and its peripheral devices for 1MW spallation neutron source including the target vessel, a mercury circulation system, and a target trolley will be reported.
